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Sustainable mix design for liquid radioactive waste with an extremely high boron concentration using alkali-activated Portland-limestone cement

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Abstract

The radioactive waste cementation plant at Paks Nuclear Power Plant in Hungary solidifies liquid radioactive waste using Portland cement blends. Under the European Green Deal, Portland-limestone cements are expected to become increasingly important due to their lower carbon footprint. However, these cements are generally unsuitable for solidification of radioactive waste with high borate concentration. This work investigates the applicability of alkali-activation for the solidification of evaporator residues with extremely high borate concentrations using Portland-limestone cement. Surface cracking was reduced using polypropylene microfibres and zeolite, resulting in stable and readily available mix designs fulfilling all technological and waste acceptance criteria.
Original languageEnglish
Pages (from-to)4881-4896
Number of pages16
JournalJournal of Radioanalytical and Nuclear Chemistry
Volume335
Issue number7
Early online date23 Jun 2026
DOIs
Publication statusPublished - Jul 2026

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

  1. SDG 3 - Good Health and Well-being
    SDG 3 Good Health and Well-being

Keywords

  • Radioactive waste
  • Portland-limestone cement
  • Solidification
  • Cementation
  • Alkali-activation
  • Zeolite
  • Fibre reinforcement

ASJC Scopus subject areas

  • Analytical Chemistry
  • Nuclear Energy and Engineering
  • Radiology Nuclear Medicine and imaging
  • Pollution
  • Spectroscopy
  • Public Health, Environmental and Occupational Health
  • Health, Toxicology and Mutagenesis

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